Kane netted a fine brace as Tottenham dismantled Everton in the Premier League on Monday night.
It moved the England captain past Henry and to within one goal of Frank Lampard's tally.
Kane has said in the past that he has his sights set on breaking Alan Shearer's incredible record of 260 goals.
He still has the best part of ten years to keep scoring in the top-flight and his form this year suggests he'll be finding the back of the net on a regular basis.
Kane now has the top five on the all-time Premier League charts in his sights but who else makes the list behind main man Shearer?
talkSPORT.com has had a look at the stellar list of names…
10. Michael Owen (Liverpool, Newcastle, Manchester United, Stoke) - 150
9. Jermain Defoe (West Ham, Tottenham, Portsmouth, Sunderland, Bournemouth) - 162
8. Robbie Fowler (Liverpool, Leeds, Man City, Blackburn) - 163
7. Thierry Henry (Arsenal) - 175
6. Harry Kane (Tottenham) - 176
5. Frank Lampard (West Ham, Chelsea, Man City) - 177
4. Sergio Aguero (Man City) - 184
3. Andy Cole (Newcastle, Manchester United, Blackburn, Fulham, Man City, Portsmouth, Sunderland) - 187
2. Wayne Rooney (Manchester United, Everton) - 208
1. Alan Shearer (Blackburn, Newcastle) - 260